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Ultrafast Spectroscopy Symposium

Join us in on 24th January 2025 for a FREE one-day workshop on Ultrafast spectroscopic techniques. In conjunction with the Warwick Centre for Ultrafast Spectroscopy (WCUS), this event aims to allow students to get the most out of the techniques and learn best practices from technical and academic experts, as well as an opportunity to share how these techniques have enabled their research.

The event is being held at Scarman, University of Warwick, open to all and is FREE to attend.

We have talk slots available for PhD students - please contact Jack and Chris with an abstract and title. (jack.woolley@warwick.ac.uk christopher.waldron@warwick.ac.uk).

Schedule:

  • Registration and Refreshments – 9:30-10:00
  • Opening and Welcome Dr Chris Waldron, Dr Jack Woolley, Warwick University - 10:00-10:10
  • Technical Talk Dr Greg Greetham, Ultra Central laser Facility: Ultrafast Spectroscopy at the Central Laser Facility - 10:10-11:00
  • Contributed Talk, Dr Edward Butler-Caddle, University of Warwick: Time resolved spectroscopy of semiconductors for photovoltaics - 11:00-11:15
  • Contributed Talk, Xinyun Liu, University of Manchester: Exploring the optoelectronic properties of Ge1-xSnx thin film heterostructures via THz spectroscopy – 11:15-11:30
  • Coffee Break, 11:30-12:00
  • Academic Talk, Dr Joseph Beames, University of Birmingham:  Spectroscopy of novel organic and inorganic emitters: Towards rational spectroscopic design - 12:00-12:45
  • Lunch - 12:45-14:00
  • Technical Talk, Dr Jack Woolley, University of Warwick: Warwick Centre for Ultrafast Spectroscopy 14:00-14:30
  • Contributed Talk, Sourav Das, University of Warwick: Optimal quantum light spectroscopy - 14:30-14:45
  • Academic Plenary, Dr Jessica Boland, University of Manchester: Helicity-dependent terahertz emission from topological insulators - a novel controllable THz source? - 14:45-15:30
  • Wrap-up - 3:30

To register, please follow the Eventbrite link

Dr Greg Greetham, Ultra Central laser Facility: Ultrafast Spectroscopy at the Central Laser Facility

ULTRA is one of the Central Laser Facility’s laboratories at the Rutherford Appleton Laboratories, focussing on time-resolved and non-linear spectroscopies. This is an open access facility for academia and industry, with applications in a wide range sciences from biomolecular dynamics to heterogeneous catalysis. An overview of the facility will be given, highlighting some of the science and technical developments at the facility. Current technical developments are focussed on HiLUX, a UKRI infrastructure funded project to install the next generation of ultrafast spectroscopy laboratories.

Dr Joseph Beames, University of Birmingham: Spectroscopy of novel organic and inorganic emitters: Towards rational spectroscopic design

Emissive chemical species are now essentially ubiquitous in our daily lives, found in everything from our lights, watches, phones to our mirrors and fridges (pretty much anything with ‘smart’ in the name). These applications are afforded by the chemical synthesis of carefully tuned organic and inorganic emitters that have precise spectroscopic emission profiles, emission lifetimes and emission quantum yields. This talk presents a combined experimental and computational chemistry insight into the use of small chemical substitutions of organic frameworks to modify photophysical properties towards those desirable for commercial applications, for example precisely tuning emission maxima in iridium complexes and enhancing triplet harvesting in organic emitters. More specifically my group use a range of laser-based techniques to probe the ground and excited state solution phase spectroscopies of these compounds alongside investigations of their excited state dynamics, complemented by ab initio computational approaches to model spectra, examine electronic transitions and predict non-adiabatic dynamics. In collaboration with several synthetic chemists, these data are used to assist in chemically modifying these emitters to rationally tune their photophysical properties. The spectroscopic datasets we generation are examined and discussed using many of the small molecule approaches that are employed within the Lester group, for example considerations of orbital symmetry and degeneracy, hindered internal rotations and computational spectral prediction.

Phosphorescence spectra of substituted Ir(III) quinoxaline complexes, some of which demonstrate impressive light upconversion quantum yields of >39% in the presence of diphenylanthracene (triplet-triplet annihilation upconversion).

Dr Jessica Boland, University of Manchester: Helicity-dependent terahertz emission from topological insulators - a novel controllable THz source?

Topological insulators (TIs) are promising candidates for a range of applications, in defense, security, imaging and telecommunications . Their topological nature provides highly-conductive surface, spin-polarised currents that are impervious to backscattering from impurities. These currents are particularly promising for applications in low-loss electronics, spintronics and quantum technologies. Here, we demonstrate that these helicity-dependent photocurrents can also helicity-dependent terahertz emission. Utilising the fantastic ultrafast photonic capability at WCUS, we demonstrate THz emission from topological insulator bismuth telluride thin films with varying bulk carrier mobility and carrier concentration. These results demonstrate that topological insulators form promising candidates for optically-switchable terahertz sources that can offer polarisation control - a key prerequisite for terahertz telecommunications.
We also show that the underlying optoelectronic properties, particularly the bulk carrier density, can have a significant impact on the THz emission properties. Optimising growth parameters to reduce the bulk carrier density can therefore improve THz emission performance further.

For any enquiries, please email the team at wasc@warwick.ac.uk and keep an eye on our Twitter for updates @WASC_Warwick

Register Here!

24th January 2025

FREE to attend

Scarman House,

University of Warwick

Coventry

CV4 7SH