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Ultrafast & Terahertz Photonics Group

Research areas

Nanomaterials

We use pump/probe spectroscopy to study how light and matter interact on femtosecond to nanosecond timescales. Using visible probes we can track electronic processes, while infrared radiation lets us study vibrational states of molecules and atomic-scale defects in semiconductors.

CNT

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Terahertz medical imaging

Performing in vivo studies of the THz properties of skin is a major initiative in the group, supported by the EPSRC Terabotics Programme GrantLink opens in a new window. We develop robust measurement protocols and test them on a statistically significant number of patients, cross-checking with other methods.

Medical

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Semiconductors and Energy materials

A major strand of our research is to improve our knowledge of the fundamental science underpinning new semiconductor materials, such as metal-halide perovskites, which are often attractive for photovoltaic applications.

Electronically-delayed optical pump/THz probe spectroscopy on a variety of semiconductors

Recent papers:

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Terahertz components, methods and techniques

We develop new THz devices and integrate them into novel systems designs that can perform THz imaging and THz spectroscopy faster, and with increased capabilities (e.g. polarisation control; robot-controlled probes).

Single-pixel

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Recent publication highlights [filter by topic: view all | highlights | THz | perovskites | nano | biomedical]

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Tracking a hysteretic and disorder-broadened phase transition via the electromagnon response in improper ferroelectrics

C. D. W. Mosley, D. Prabhakaran and J. Lloyd-Hughes
J. Phys. D: Applied Physics 51 084002 (Jan 2018) [ pdf ][ ref ]

We demonstrate that Hysteresis in the electromagnon oscillator strength in CuZnOelectromagnons can be used to directly probe the nature of a phase transition between magnetically ordered phases in an improper ferroelectric. The antiferromagnetic/paraelectric to antiferromagnet/ferroelectric phase transition in Cu1-xZnxO (x = 0, 0.05) alloys was tracked via the electromagnon response using terahertz time-domain spectroscopy, on heating and cooling through the phase transition. The transition was found to exhibit thermal hysteresis, confirming its first-order nature, and to broaden under the influence of spin-disorder upon Zn substitution. The energy of the electromagnon increases upon alloying, as a result of the non-magnetic ions modifying the magnetic interactions that give rise to the multiferroic phase and electromagnons. We describe our findings in the context of recent theoretical work that examined improper ferroelectricity and electromagnons in CuO from phenomenological and first-principles approaches.

Wed 17 Jan 2018, 08:02 | Tags: THz spectroscopy, 2018, Lloyd-Hughes

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