Ultrafast & Terahertz Photonics Group
Ultrafast optical techniques provide powerful probes of different states of matter, using light pulses that have femtosecond duration. In Warwick our activities span a number of areas:
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Group facilitiesThe Group has labs across the campus, in the main Physics building, Materials and Analytical Sciences, and Millburn House. Read more about our experimental capabilities in terahertz science and technology. We also run the Warwick Centre for Ultrafast Spectroscopy Research Technology Platform. We make use of a wide range of Warwick's excellent materials analysis equipment, including X-ray diffraction, Raman spectroscopy, electron microscopy and magnetometry. |
Join the group!We have funded PhD positions available to work on nanoscale imaging of perovskitesLink opens in a new window, coherent vibrations of defect in diamond, Link opens in a new window THz sensing for biomedical applicationsLink opens in a new window and ultrafast studies of battery materialsLink opens in a new window. These are available for UK students and potentially for exceptional international students. Please get in touch if you are interested in PhD or MSc by Research topics in the group. We are also happy to support postdoctoral researchers to apply for fellowship schemes. Group, Theses & PhotosContact details for our current group members and our photo gallery. For recent theses from the group, please see here. |
Research areas
Nanomaterials
We use pump/probe spectroscopy to study how light and matter interact on femtosecond to nanosecond timescales. Using visible probes we can track electronic processes, while infrared radiation lets us study vibrational states of molecules and atomic-scale defects in semiconductors.
Recent papers:
Quantifying photoluminescence variability in monolayer molybdenum disulfide films grown by chemical vapour deposition
The 3237 cm−1 diamond defect: Ultrafast vibrational dynamics, concentration calibration, and relationship to the N3VH0 defect
Terahertz medical imaging
Performing in vivo studies of the THz properties of skin is a major initiative in the group, supported by the EPSRC Terabotics Programme GrantLink opens in a new window. We develop robust measurement protocols and test them on a statistically significant number of patients, cross-checking with other methods.
Recent papers:
Effect of transdermal drug delivery patches on the stratum corneum: in vivo inspection with a handheld terahertz probe
Terahertz probe for real time in vivo skin hydration evaluation
Spectroscopic insight on impact of environment on natural photoprotectants
Semiconductors and Energy materials
A major strand of our research is to improve our knowledge of the fundamental science underpinning new semiconductor materials, such as metal-halide perovskites, which are often attractive for photovoltaic applications.
Recent papers:
Distinguishing carrier transport and interfacial recombination at perovskite/transport-layer interfaces using ultrafast spectroscopy and numerical simulation
Temperature-Dependent Structural and Optoelectronic Properties of the Layered Perovskite 2-Thiophenemethylammonium Lead Iodide
Terahertz Emission via Optical Rectification in a Metal-Free Perovskite Crystal
Terahertz components, methods and techniques
We develop new THz devices and integrate them into novel systems designs that can perform THz imaging and THz spectroscopy faster, and with increased capabilities (e.g. polarisation control; robot-controlled probes).
Recent papers:
Simultaneous measurement of orthogonal terahertz fields via an emission multiplexing scheme
Optimum Optical Designs for Diffraction-Limited Terahertz Spectroscopy and Imaging Systems Using Off-Axis Parabolic Mirrors
The 2023 terahertz science and technology roadmap
Recent publication highlights [filter by topic: view all | highlights | THz | perovskites | nano | biomedical]
Resolving the Ultrafast Charge Carrier Dynamics of 2D and 3D Domains within a Mixed 2D/3D Lead-Tin Perovskite
Jake D. Hutchinson, Edoardo Ruggeri, Jack M. Woolley, Géraud Delport, Samuel D. Stranks, Rebecca L. Milot
Advanced Functional Materials 2305736, (August 2023)
Ultrafast THz spectroscopy of carbon nanotube-graphene composites
M.G. Burdanova, A.P. Tsapenko, S. Ahmad, E.I. Kauppinen and J. Lloyd-Hughes
Nanotechnology 34 405203 , (June 2023)
Spectroscopic Insights into the Influence of Filling Carbon Nanotubes with Atomic Nanowires for Photophysical and Photochemical Applications
Z. Hu, B. Breeze, M. Walker, E. Faulques, J. Sloan and J. Lloyd-Hughes
ACS Appl. Nano Mater. 6, 2883 (Feb 2023)
Terahertz photoconductance dynamics of semiconductors from sub-nanosecond to millisecond timescales
E. Butler-Caddle, N.E. Grant, S.L. Pain, J.D. Murphy, K.D.G.I. Jayawardena and J. Lloyd-Hughes
Appl. Phys. Lett. 122 012101 (Jan 2023)